By A. Schuster, J. Nicholson
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The dispersion measurements for SY215 were performed using dichloromethane (CH2CI2) as the solvent due to the vibrational overtones of dioxane and the potential absorption of the molecule at the second harmonic. The linear optical absorption spectrum of SY215 in CHjC^ is shown in Fig. 9. The visible peak at 688 nm, is red-shifted compared to that in 1,4-dioxane (632 nm) due to the solvatochromic effect. The absorption peak is also wider. Again, seven wavelengths have been selected for the dispersion measurement, ranging from 1600 nm to 1960 nm.
1960, 32, 140. ; ACS Symposium Series; American Chemical Society: Washington, DC, 1995. Chapter 3 Hyperpolarizabilities of Push—Pull Polyenes Molecular Orbital and Valence-Bond Charge-Transfer Models 1,2 1,2 2,3 2 2 J. W. Perry , S. R. Marder , F. Meyers , D. Lu , G. Chen , W. A. Goddard, III , J. L. Brédas , and B. M. O. Box 92426, Los Angeles, CA 90009-2426 2 3 4 In this paper we review two theoretical approaches that illustrate the relationships between molecular (hyper)polarizabilities and bondlength alternation (BLA).
ACS Symposium Series; American Chemical Society: Washington, DC, 1995. 38 POLYMERS FOR SECOND-ORDER NONLINEAR OPTICS the relatively strong absorption comingfromthe overtone of 1,4-dioxane (20) peaking at around 1700 nm. The slight discrepancy between theory and experiment at high photon energies may be attributed to the inability of the theory to reproduce the oscillator strength of the second major absorption peak. The presence of the second absorption peak resulting from the S - » S transition will very likely increase the slope of the dispersion.